Chem 334
Spring 2010

Professor Joseph M. Fox
272 Brown Labs
302-831-0191
jmfox@udel.edu
Labs are held in Rm 318 Drake
Office hours: Mondays 11-12, or by appointment.  Contact me by email to schedule an appointment



Teaching Assistants for this course
Danielle McAtee, dmcatee@udel.edu
Anil Pandey, pandey@UDel.Edu
Sha Bai, baisha@UDel.Edu

Sections for this course

Section 010: Monday 12:20PM - 3:20PM,  Tuesday 12:30PM - 3:30PM, TA=McAtee
Section 011: Monday 3:35PM - 6:35PM, Tuesday 3:30PM - 6:30PM, TA=Pandey
Section 012: Monday 7:00PM - 10:00PM, Tuesday 7:00PM - 10:00PM. TA=Bai


Safety
You Must Have Safety Goggles
No Shorts
No Open Toed Shoes
No Food or Drink
Come Prepared, Read the Assignment, and Bring your Notebook
Textbooks:
Organic Chemistry Laboratory, Third Edition by Bell, Clark and Taber

Learning Goals for this Course

Through successful completion of this course:
1) Students will learn safety procedures in the organic lab
2) Students will learn how to document experiments in a notebook
3) Students will learn how to interpret material safety data sheets
4) Students will know how to setup and analyze a diverse range of organic chemistry experiments, monitor their progress, purify products, and analyze their purity.
5) Students will learn how to purify products using crystallization, distillation, column chromatography
6) Students will learn how to analyze spectral data using IR spectroscopy, 1H NMR spectroscopy, 13C NMR spectroscopy,  and polarimetry.
7) Students will learn how to determine the purity of substances using TLC, melting point analysis in addition to the above spectral techniques
8) Students will develop an appreciation for green chemistry through experiments
9) Students will learn how to use spectroscopy to reveal the structure of an unknown substance
10) Students will participate in an independent study, wherein they research a two-step chemical synthesis.  Students will learn how to utilize chemical databases to research the scientific literature, and will use modern spectroscopic techniques to determine the successfulness of their independent projects.

Links:

Chem 332 Spring 2010
Chem 332 Spring 2009
Chem 332 Spring 2008
Chem 332 Spring 2007
Chem 332 Spring 2006
Chem 332 Spring 2005
Chem 332 Spring 2003


Chem 334 Spring 2009
Chem 334 Spring 2008
Chem 334 Spring 2006
Chem 334 Spring 2005
Chem 334 Spring 2003


Prof. Taber's course page for Chem 334 (previous years)
Chem 333

Chemical Database Searching Tutorials

Intro to Beilstein Handout from Chem 333 (Dr. Koh,  lab 7)

<>The following handouts demonstrate how to do more advanced searches with Beilstein.  Although they show the old Beilstein interface, the concepts are the same with the new interface.  Especially important (for the independent study) is the reaction searching using substructures

Handout: Introduction to substructure searching on Beilstein Commander
Handout: Introduction to Reaction searching with substructures on Beilstein commander

Powerpoint presentations:
IR handout
Mass Spec and UV-Vis handout

Grading
There will be a lab exam that will constitute 33% of your grade. The rest of your grade will be based on your lab grade (34%) and on your performance in the independent study (33%). Before each lab, you will be given a short (5 min) quiz by your TA, in which you will demonstrate your preparedness. You will turn in your notebook at the end of each lab period. Your TA will grade it and return it to you promptly.
 

Handouts
As needed to supplement the text will be posted on the course Web site.
 

Lab Exams
A Lab exam will be given (time and date TBA).    Those in the Honors section must also take the lab exams.  The Exams will cover spectroscopy and structure elucidation, and will be open book and open notes.  Be sure to study exam questions from earlier years (see links below).


Exam 1 2010     Answers to Exam 1 2010


Prior year's lab exams

Exam 1 2009     Answers to Exam 1 2009

Exam 2 2009     Answers to Exam 2 2009


Exam 1 2008     Answers to Exam 1 2008

Exam 2 2008       Answers to Exam 2 2008


Exam 1 2007       Answers to Exam 1 2007

Exam 2 2007       Answers to Exam 2 2007

Final Report for the Independent study
The report for the independent study must be typed, and it roughly follows the format for a full paper written to an American Chemical Society journal.   Chemical structures (and reagents that accompany those structures) may be drawn by hand.  Presentation, grammar, spelling and writing style will count!  Your final report is worth 50 points (to be averaged with the points that you receive from your TA).  The independent study will be initially reviewed by your TA, and then graded by me.  Please turn your report in to your TA on Friday,

 29th.  Revisions may be neccessary, and will be due one week after it is returned to you.

Sections of the report:

Introduction: Write a brief introductory statement (license to use your creative writing skills here).  Using chemical structures, show the reaction that you carried out.  Provide references in the following format: Authors, "Title of Article" Journal Name Year, Volume Number, pages.  You should also detail the accepted mechanism for each of the reactions that you studied.

Results and Discussion: Briefly explain what you did experimentally, and if you consider the experiment to have been successful.  While reagents and reaction times are appropriate for discussion, don't talk about all of the nitty gritty details.  Do elaborate on any differences between what you did and what was published. Unless they are of special importance, leave out discussion of filtering procedures, volumes of solvents, and work up procedures.  State if your product was purified by chromatography, but don't tell me the chromatography solvents or the number of test tubes that you collected.  Basically, in this section you describe and discuss what you found without boring us with the details.  We can find those in your lab notebook pages.

Discuss details of how the spectroscopic information supports the assignment of your structure, the purity of the material, etc.  It should not be a description of every single data point.  For IR data, you should discuss peaks associated with major functional groups.  For example, pointing out that your ketone product has a peak at 1715 cm–1 in the IR spectrum is important information.  Similarly, pointing out that you observed a peak at 202 ppm in the 13C NMR would also be relevant  for discussion.  Any other information that serves to support your findings (e.g. melting point in agreement with the literature; TLC evidence ; color of the compound is in agreement with the literature) should also be discussed. 

For NMR data, you should provide tables with detailed peak assignments, including a discussion of multiplicity.

Conclusions: Tell us if your reactions worked, and if they would be suitable for incorporation into the regular undergraduate  lab.  Briefly support your statements.

Supporting Information: Provide an appendix with hard copies of any spectra (NMR, IR, etc); provide copies of the articles that you used.  Also, please photocopy the pages from your lab notebook and include those pages in the appendix.

 

Protective Equipment
Goggles are required and must be worn at all times in the laboratory. Suitable clothing must also be worn.
 
 

0 Week of Feb. 8 - Develop a plan for your Independent Study project.  Use Beilstein to find suitable precedent.  You need to turn in a copy of the articles that you wish to adapt.  Follow the guidelines set forth on the following checklist (for an example, see this sample checklist)

1 Week of Feb 15:
    Session 1, Beilstein TA office hours in 222 BrL.  
    Session #2: Chp. 37 A1, A2 Heterocycle Synthesis, p 293-5.  Start Benzopinacol

NOTE: Proposed Independent Study due to your TA in the first lab session of Monday Feb 22th 

2 Week of Feb 22; 
    Session 1,
Finish Benzopinacol
    Session #2: Ester Hydrolysis–recycling polyethylene terephthalate; Start Orange Peel Esterase

3  Week of Mar 1.
    
   Session #1: Finish Orange Peel Esterase
    Session #2:   Biofuel
4
Week of Mar 8

    Session #1: BCT chapter 40, page 309 Resolution of alpha-phenylethylamine
    Session #2: continue  Resolution of alpha-phenylethylamine

5 Week of March 15
    Session #1:   unknown Suzuki
    Session #2:   unknown Suzuki

6 Week of March 22
    Session #1:   unknown Suzuki
    Session #2:    Chp. 28A Nucleophilic Aromatic Substitution, p 249-51 

Spring Break

7 Week of April 5nd Both sessions: Independent Study

8 Week of April 12th  Both sessions: Independent Study

9 Week of April 19th.  Both sessions: Independent Study

10 Week of April 26th
    Session #1:  lab does not meet--study for Lab Exam
    Session #2: Chp. 30 AB Chemiluminescence

11 Week of  May 3.  Independent study final report due to your TA at the first lab session.
    Session #1: Chp. 30 AB Chemiluminescence
    Session #2:  tropinone

12 Week of May 10
    Session #1: Beckmann rearrangement
    Session #2: Clean up, check out